I don't know about adding a password to Outlook it's self. However you can add a password to the mail store.
Open Outlook > Click on Tools > Click Options > Click Mail Setup Tab > Click Data Files button > Hilight your mail store file (There should only be one) > Click on the settings button > Click on Change Password button > Leave the current password text box blank > add your password to the other boxes > Make sure that you leave the Save This Password to your Password List unticked > Click OK or Close to get back to the Outlook screen.
Now each time you open outlook you will be prompted for a password.
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